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Ursula Keller wins “Swiss Nobel” Marcel Benoist Prize- for pioneering work in ultrafast lasers
MUST2022 Conference- a great success!
New scientific highlights- by MUST PIs Wörner, Chergui, and Richardson
FELs of Europe prize for Jeremy Rouxel- “Development or innovative use of advanced instrumentation in the field of FELs”
Ruth Signorell wins Doron prizefor pioneering contributions to the field of fundamental aerosol science
New FAST-Fellow Uwe Thumm at ETH- lectures on Topics in Femto- and Attosecond Science
International Day of Women and Girls in Science- SSPh asked female scientists about their experiences
New scientific highlight- by MUST PIs Milne, Standfuss and Schertler
EU XFEL Young Scientist Award for Camila Bacellar,beamline scientist and group leader of the Alvra endstation at SwissFEL
Prizes for Giulia Mancini and Rebeca Gomez CastilloICO/IUPAP Young Scientist Prize in Optics & Ernst Haber 2021
Nobel Prize in Chemistry awarded to RESOLV Member Benjamin List- for the development of asymmetric organocatalysis
NCCR MUST at Scientifica 2021- Lightning, organic solar cells, and virtual molecules

Attosecond pump-probe setup

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Location Contact
ETH Zurich
Wolfgang-Pauli-Str. 10
HCI G222
8093 Zurich
 
 Martin Huppert
Tel +41 44 633 4368
7mac-rtb-inq1.hj)uph6peg0rte$@pl5hye*s.l3cht4emd#.em9thv%z.y)chz
 

Setup / Configuration

  • XUV/IR or XUV/UV-VIS delay line
  • Piezo driven delays from 10 as to 3 ps
  • Active stabilization with kHz bandwidth
  • Stability in the 10 as range
  • Absolute path length detection
  • XUV and IR beams can be modified separately (spectral filtering, polarization control, frequency conversion)
  • Overall XUV reflectivity ~ 40%
  • (30-150 eV)                                           
 

Literature

  • M. Fieß, M. Schultze, E. Goulielmakis, B. Dennhardt, J. Gagnon, M. Hofstetter, R. Kienberger and F. Krausz, Versatile apparatus for attosecond metrology and spectroscopy“, Rev. Sci. Instrum. 81, 093103 (2010).
  • M. Holler, “Attosecond strong field control”, Ph.D. Thesis, ETH Zürich, Nr. 18782, 2010.
  • F. Schapper, “Attosecond structure of high-order harmonics”, Ph.D. Thesis, ETH Zürich, Nr. 18783, 2010.

                           

W11

w2

The top image shows the design of the attosecond interferometer using a semi-infinite gas cell as XUV source and a velocity-map imaging (VMI) spectrometer as detector. The bottom image shows the realization in our laboratory.  
 Our setup generates a controlled attosecond delay between two ultrashort pulses: an infrared or ultraviolet and an extreme-ultraviolet (XUV) pulse. The attosecond interferometer represents a versatile tool to realize pump-probe measurements of electronic dynamics in polyatomic molecules. It can be combined with an XUV spectrometer for transient absorption measurements, a VMI spectrometer for angle-resolved photoelectron measurements or with a photoelectron time-of-flight spectrometer for liquid samples.
We are using a sophisticated stabilization scheme to stabilize the interferometer to arbitrary delays. The feedback loop using interferences of a He-Ne laser beam is realized fully digitally in a real-time computer system, which allows loop rates in the kilohertz range. In addition, a white-
light interferometer gives information about the absolute path length difference between the two arms of the interferometer.


 
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